'Chloë and the Next 20th Century' was written and recorded between August and December 2020 and features arrangements by Drew Erickson. The album sees Tillman and producer/multi-instrumentalist Jonathan Wilson resume their longtime collaboration, as well as Dave Cerminara, returning as engineer and mixer. Basic tracks were recorded at Wilson's Five Star Studios with strings, brass and woodwinds recorded at United Recordings in a session featuring Dan Higgins and Wayne Bergeron, among others.
 
Bella Union - BELLA1274VB